放射性核素在处置库屏障材料上吸附行为国内研究进展

    China’s Research Advances in Radionuclides Sorption on Repository Barrier Materials

    • 摘要: 放射性废物的处置问题是制约我国核能可持续发展的主要因素之一。虽然不同类型的放射性废物对应不同的处置方式,但均需通过核素迁移研究进行处置安全评价。吸附作用是控制放射性核素在处置体系中迁移行为的关键过程,也是处置库安全评价的核心研究内容。本文首先概述了处置库关键屏障材料、吸附研究方法、吸附机理和吸附建模思路。继而从吸附实验和模型构建进展两个方面,梳理并评述了近二十年来国内学者取得的研究成果。最后,对我国未来放射性废物处置背景下的吸附研究做了展望。

       

      Abstract: The disposal of radioactive waste is one of the major factors constraining the sustainable development of nuclear energy in China. Although different types of radioactive waste correspond to different disposal methods, safety assessment for disposal in all cases must be carried out through research on radionuclide migration. Sorption is a key process governing the migration behavior of radionuclides within the disposal system, and consequently forms a core research topic for evaluating disposal safety of radioactive waste. This paper first outlines the key barrier materials in repositories, research methodologies for sorption, sorption mechanisms, and approaches to adsorption modeling. It then reviews and evaluates the research achievements made by domestic scholars over the past two decades, focusing on progress in sorption experiments and adsorption modeling. Finally, prospects and suggestions are proposed for future sorption research in the context of radioactive waste disposal in China.

       

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