未辐照快堆(U,Pu)O_2燃料的溶解试验

    • 摘要: 研究了未辐照UO_2、(U,Pu)O_2燃料在硝酸中的溶解行为。详细描述了硝酸浓度、温度、芯块加工方法和PuO_2含量等因素对溶解速度的影响,测定了溶解过程中钚价态变化和难溶残渣含量。

       

      Abstract: DISSOLUTION OF UNIRRADIATED LMFBR(U,PU)O_2FUELZHANG SHAOQI;WEI XIUFANG;HOU XIAOLIN(China Institute of Atomic Energy,P.O. Box 275,Beijing,102413)WANG SHOUXIN;GAO YAOBIN;CHENG QINCHENG(Lan Zhou Nuclear Fuel Complex,P.O.Box 508,732850)ABSTRACT Dissolution behaviour of unirradiated LMFBR(U,Pu)O_2 fuel in HNO_3 is studied.Theeffects of HNO_3 concentration,dissolution temperature(U,Pu)O_2 pellet fabrication method(mechanical blending and AUPUC coprecipitating)and PuO_2 content on dissolution rate aredescribed in detail. The content of undissolved residues and the percentage of Pu(Ⅵ)in dis-solution solution are determined. Key words Fuel dissolution UO_2(U,Pu)O_2

       

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