放化法测量~(79)Se的半衰期

    • 摘要: 长寿命裂变产物核素 ̄(79)Se的半衰期还没有被准确地测量过,文献中一直引用1949年测定的值:T_(1/2)≤6.5×10 ̄4a。本工作应用放化法测量了 ̄(79)Se的半衰期。从中子照射的铀靶中分出放化纯的 ̄(79)Se,并用液闪谱仪测量其活度。利用 ̄(90)Sr、 ̄(137)Cs作为监测核计算出铀靶的裂变数,然后根据裂变产额得到 ̄(79)Se核数。得到的 ̄(79)Se的半衰期为(4.8±0.4×10 ̄5a。)

       

      Abstract: MEASUREMENT OF HALF LIFF OF ~(79)Se USING RADIOCHEMICAL METHODYU RUNLAN;GUO JINGRU;CUI ANZHI;TANG PEIJIA; LI DAMING;LIU DAMING(China Institute of Atomic Energy,P,O,Box 275(26),Beijing 102413)ABSTRACT~(79)Se is a long lived fission product nuclide. Scientists gradually pay attention to ~(79)Se owing toits importance in radiowaste disposal.Its half life value must be known accuratelv in order to cal-culate its content in radiowaste and the radiation dose of ~(79)Se migrated to biosphere. Up to now,however,there is no accurate value inkerature, In 1949 Parker et al.measured the half life of ~(79)Se,but they only obtained an upper limit,T_(1/2)≤6.5×10~4a,which is still used at present in nu-dear data literatureq. In the present work,the half life of ~(79)Se has been measured using radioChemical method.Ra-diochemically pure ~(79)Se is separated from irradiated ~(235)U targets and its activity is measured by aliquid scintillation spectrometer. According to its fission yield the number of’9Se nuclei is calculat-ed by means ofhsion monitors.~(137)Cs and ~(90)Sr are selected as monitors. The activitv is measuredusing HPGe γ spectrometer for ~(137)Cs and Cherenkov liquid scintillation counting for ~(90)Sr. The halflife of ~(79)Se is obtained to be(4.8±0.4)×10~5a. Key words ~(79)Se Half fife Fission monitors.

       

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