计算机模拟法研究铀钚的非还原分离

    • 摘要: 应用遗传算法研究了铀钚的非还原分离,得到了一个可行的工艺条件,计算了该工艺条件下U(Ⅵ)、Pu(Ⅳ)和酸的浓度剖面,分析了各变量的灵敏度和操作弹性。计算结果表明,用稀酸可以实现铀钚的非还原分离,同时得到铀产品及不同钚浓度的制备MOX元件的铀钚混合液。

       

      Abstract: STUDY ON THE NONREDUCTIVE SEPARATION OF U AND Pu USING SIMULATING METHODHan Binbing Wu Qiulin Zhu Yongjun(Institute of Nuclear Energy Technology,Tsinghua University,P.O.Box 1021,Beijing 102201)ABSTRACTThe nonreductive separation of U(Ⅵ) and Pu(Ⅳ) is studied using genetic algorithm. A possible process is proposed. The yields of U in organic stream and Pu in aqueous stream are above 99.8%. The sensibility of the yield and content of both U(Ⅵ) and Pu(Ⅳ) in every stream are obtained. Operation flexibility of each parameters is demonstrated. The results of calculation show that the nonreductive separation of U and Pu can be obtained using diluted acid stripping. In this proposed process,the pure U product and UPu mixture for preparation of MOX fuel can be obtained simultaneously.Key words NonReductive separation Genetic algorithm Sensibility Operation flexibility

       

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