大气气溶胶含碳组分的来源研究──加速器质谱法

    • 摘要: 使用加速器质谱(AMS)技术进行了大气中气溶胶含碳组分的来源分析。对于北京近郊区采集的总悬浮颗粒物(TSP)样品,多元统计模式计算结果表明,TSP的最主要来源是土壤扬尘,对大气气溶胶的贡献超过了50%。然而,AMS技术分析结果显示,大气气溶胶的含碳组分与微量元素组分有十分显著的来源差异。北京(非采暖期)、湖南南岳镇和山东青岛的气溶胶含碳组分中,来自矿物燃料人为燃烧的贡献大约占70%,随着人为活动的增加,这一比例还会增加。

       

      Abstract: STUDY ON SOURCE IDENTIFICATION FOR CARBONACEOUS AEROSOLS──THE APPLICATION OF ACCELERATOR MASS SPECTROMETRYShao Min;Li Jinlong;Tang Xiaoyan(State Joint Key Laboratory of Environmental Simulation and Pollution Control,Center of Environmental Sciences, Peking University,Beijing100871)Wang Jianjun;Guo Zhiyu;Liu Kexin;Lu Xiangyang;Li Bin;Li Kun (Institute of Heavy Ion Physics,Peking University,Beijing100871)Abstract:The study on source identification for atmospheric carbonaceous aerosols by accelerator mass spectrometry is described.For comparison,the source of trace elements in aerosols by multivariate analysis models is studied.For the samples collected in suburb of Beijing,the results by factor analysis show that the predominant TSP source was soil which contributes more than 50%to atmospheric aerosols,However,the AMS results demonstrate that carbonaceous aerosols have quite different emission sources,For carbonaceous aerosols of Beijing,Hunan and Shandong,the contribution to ambient particles from fossil fuel is nearly 70%,and as the man-made activities(such as coal-burning)increase,the fossil burning will have more contributions.Keywords: AMS Aerosol Factor analysis Source identification

       

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