~(235)U热(慢)中子裂变碎片在水中的射程
RANGES OF THE FRAGMENTS FROM THERMAL (SLOW) NEUTRON FISSION OF ~(235)U IN WATER
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摘要: 根据厚靶原理,用各种浓度的氯化铀酰水溶液作为厚靶,用已确定表面积的铂片作为吸收体浸没于铀溶液中,测定热(慢)中子引发~(235)U裂变碎片~(89)Sr,~(91)Y,~(140)Ba,~(141)Ce,~(144)Ce在各铀浓度的水溶液中的射程值。在含铀量为0.16%—6.2%的范围内,铀浓度对射程测定值没有明显影响。因此,可以认为当铀溶液足够稀时,裂片在铀溶液中的射程很接近于它们在水中的射程。实验得出该五种裂片在水中的射程分别为:R_(Sr-90)=2.39+0.04mgcm~(-2),R_(Y-91)=2.355±0.09mgcm~(-2),R_(Ba-140)=1.92+0.07mgcm~(-2),R_(Ce-141)=1.91±0.12mgcm~(-2),R_(Ce-144)=1.84+0.10mgcm~(-2)。为了估计裂片在铂片中反散射的影响,进行了以不锈钢片作为吸收体的实验(用硝酸铀酰水溶液作为厚靶),结果表明反散射的影响不大。本工作为测定裂片在液体中的射程提供了一个较简便的方法。Abstract: Acccording to the principle of thick target, we used the aqueous solutions of uranyl chloride of various concentrations as thick targets and platinum plates of known surface area as absorbers immersed in the target solutions. The ranges of the U(n,f) fission fragments 89Sr, 91Y, lioBa, 141Ce and 144Ce in the'aqueous solutions of uranyl chloride of various concentrations were determined. In the concentration region of 0.16 U%-6.2 U%, the uranium concentration had no significant effect on the measurement of the range. Therefore, the ranges of the fission fragments in dilute U02C12 solutions are very close to that in pure water, and the mean value of the ranges in U02C12 solutions of various concentrations was taken as the range in water. The experimental result of the ranges of these five fission fragments in water were: RSt-90 = 2.39±0.04mgcm-2, Ry-91 = 2.35±0.09mgcm-2, RBa-140 = 1.92±0.07mgcm-2, RCo-141=1.91±0.12mgcm-2, Rc0-144=1.84±0.10mgcm-2. In order to estimate the effect of back scattering of fission fragments in platinum plate, we did the experiments using stainless steel plate as absorber (the aqueous solutions of uranyl chloride as thick targets). The results were similar. Thus, the effect of back scattering was not significant. This work provides a convenient means for determining the ranges of the fission fragments in a liquid.