~(252)Cf自发裂变中子诱发~(235)U裂变时几个核素裂变产额的绝对测定

    THE ABSOLUTE DETERMINATION OF CUMULATIVE YIELD OF SEVERAL NUCLIDES FROM INDUCED FISSION OF ~(235)U BY NEUTRONS OF SPONTANEOUS FISSION OF ~(252)Cf

    • 摘要: <正> 引言 在燃耗测量工作中,常应用质量产额曲线峰上的裂变产物核素作为监测体。一般说来,这些核素的裂变产额随入射中子能量的变化不灵敏。但是~(99)Mo的情况比较复杂。文献中~(235)U热中子裂变的产额数据相互符合得较好,但是裂变谱或快堆谱诱发裂变时,数据比较混乱,

       

      Abstract: The cumulative yields of 95Zr, 99Mo and 147Nd in the fission of 235U induced by neutrons of spontaneous fission of 252Cf were determined absolutely by radiochemical method.In Nov. 1978, the weight of 252Cf used as the neutron source of spontaneous fission was 100 μg, which was sealed within aluminium cylinder tube. When irradiated, the distance from the targets to the neutron source was about 5 cm.The sample targets were highly enriched uranium 235U (90%). The standard targets were prepared by molecular plating and the sample targets were uranium metal disks with masses from 2 to 3 gramms.The absolute fission rate of the sample target was measured by double fission ioni-zation chamber as described in a previous paper6.The cumulative yields determined are listed in following table:The errors given in the table are total errors including statistical and systematic errors. The yield values of 95Zr, 99Mo and 147Nd in the fission of 235U induced by neutrons of spontaneous fission of 252Cf are found to be in agreement with the yields induced by fission spectrum neutrons of 235U within error limits.

       

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