239Pu(nth,f)短寿命裂变产物产额测量

    Short-Lived Fission Products Yield Measurement for 239Pu(nth,f)

    • 摘要: 采用γ能谱相对测量方法,以97Zr为内标参考核素,完成了239Pu(nth,f)短寿命裂变产物88Rb、95Y、101Mo、101Tc、138Csg142La等核素的累积产额测量。实验测得88Rb、95Y、101Mo、101Tc、138Csg142La的累积产额数据分别为(1.32±0.05)%、(4.69±0.22)%、(6.13±0.32)%、(6.10±0.22)%、(6.24±0.24)%、(4.74±0.17)%。对高纯锗探测器中高能端效率刻度、样品封装与辐照、γ谱测量几何条件设计、γ谱测量与数据分析进行了研究。实验测量裂变产物核素分别位于非对称裂变质量分布双驼峰曲线轻峰的左侧、中部和右侧,重峰的中部与右侧。

       

      Abstract: The cumulative fission yields of shortlived nuclides 88Rb, 95Y, 101Mo, 101Tc, 138Csg, and 142La in thermal neutron induced fission of 239Pu have been determined by gamma-ray spectrometry relative method. 97Zr is selected as the reference nuclide. The determined cumulative fission yields are given as following: the Y(88Rb)=(1.32±0.05) %, Y(95Y)=(4.69±0.22)%, Y(101Mo)=(6.13±0.32 )%, Y(101Tc)= (6.10±0.22)%, Y(138Csg)= (6.24±0.24)%, Y(142La)=(4.74±0.17)%. The major work include HPGe detector efficiency calibration, sample sealing and irradiation, gamma-ray measurement and data analysis. The determined nuclides are located in left, middle, right of light group, and in middle, right of heavy group for asymmetric fission model. The accurate yields data supply a gap for domestic nuclear database, and reflect the fission products mass distribution character in thermal neutron induced fission of 239Pu.

       

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