高放废液处理过程中总β放射性活度的分析
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摘要: 研究了高放废液处理过程中总β放射性活度的分析方法。用液体闪烁计数法甄别α和γ射线的干扰,测量水相和有机相总β放射性的计数率。把β放射性核素分成4组,用液闪仪和Ge(Li)γ谱仪分析各组样品和各种淬灭条件下的等效效率和权重因子,通过效率等效法计算得到样品的总β放射性活度。分析了TRPO处理生产堆高放废液流程中各液流的总β放射性活度。总β测量的不确定度小于5%。Abstract: ANALYSIS OF GROSS BETA ACTIVITY IN THE TRPO PROCESSLiang Junfu Liu Xiuqin Guo Yifei(Institute of Nuclear Energy Technology,Tsinghua University, P.O.Box 1021,Beijing 102201)ABSTRACTAnalysis of gross beta activity in the TRPO process for treating high level liquid waste is studied.The gross beta activity in aqueous or organic phase samples are determined by liquid scintillation analyzer.Interference with determination of α and γ to β is discriminated.β nuclides are divided into four groups based on β maximum energy.Equivalent efficiency and weigh factor of each group are analyzed by liquid scintillation analyzer and Ge(Li) γ spectrometer.Gross β activities of the samples are calculated by equivalent efficiency method.The method is applied to analysis of gross β activity in the TRPO process with satisfactory results.Key words Gross beta activity Liquid scintillation counting High level liquid waste Equivalent efficiency method
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[1] 1吕峰,林灿生,张先梓,等.高放废液总β放射性活度测量.原子能科学技术,1992,26(5):892罗文宗.高放废液中放射性核素分析.原子能科学技术,1992,26(5):63马崇智,等.放射性同位素手册.北京:科学出版社,1979,5594梁俊福,刘秀琴,郭一飞.萃取液闪法测定高放废液及其处理工艺中90Sr.清华大学学报,1996,36(11):865刘秀琴,梁俊福,郭一飞.萃取液闪法测定高放废液及其处理工艺中99Tc.核电子学与探测仪器,1997,17(3):1806田国新,梁俊福.TRPO处理高放废液过程中α核素的分离、测定方法.核化学与放射化学,1996,18(2):1227郭一飞,梁俊福,焦荣洲.激光荧光法测定高放废液及其处理工艺中的铀.原子能科学技术,1997,31(4):3218BeargAP.TheEficiencyExtrapolationMethodinCoincidenceCounting.NuclInstrumMethods,1973,112(1,2):143
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